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Polymers are materials with vast environmental and economic ramifications, yet are generally not discussed in secondary education science curricula. We describe a program in which college mentors develop and implement hands-on, polymerrelated experiments to supplement a standard, state regents-prescribed high school chemistry course, as well as a middle school elective course on polymers. Interactive experimentation and feedback-oriented design are highlighted as critical elements to the success of the program. The experiments have been executed in two vastly different institutions: a New York City magnet high school for underprivileged females, and a private middle school for privileged male and female students; the similarities and differences are juxtaposed